Kavli Affiliate: Frank Wise | Summary:Raman scattering underlies a broad range of spectroscopic and light-generation techniques, yet its conventional description, based on the Raman gain spectrum, accurately describes only long-pulse, steady-state dynamics. We present and develop a time-domain theoretical approach that provides a unified and physically-transparent description of Raman interactions across all temporal regimes. It […]

Kavli Affiliate: Frank Wise | Summary:Raman scattering underlies a broad range of spectroscopic and light-generation techniques, yet its conventional description, based on the Raman gain spectrum, accurately describes only long-pulse, steady-state dynamics. We present a time-domain theoretical approach that provides a unified and physically-transparent description of Raman interactions across all temporal regimes. It enables direct […]

Kavli Affiliate: Frank Wise | Summary:Raman scattering underlies a broad range of spectroscopic and light-generation techniques, yet its conventional description, based on the Raman gain spectrum, accurately describes only long-pulse, steady-state dynamics. We employ a time-domain theoretical approach to account for spectrotemporal aspects of continuous frequency-shifting, which are not addressed by prior theories. In particular, […]

Kavli Affiliate: Darrell Schlom | Summary:The prototypical Mott-Hubbard insulator LaVO3 undergoes a structural phase transition accompanied by the onset of spin and orbital ordering below 140 K. By combining ultrafast optical pump-probe spectroscopy and two-dimensional electronic spectroscopy, we investigate the interplay between fluctuations of the local spin and orbital order parameter and the lifetime of […]

Kavli Affiliate: Brad Ramshaw | Summary:The candidate topological superconductor UTe$_2$ exhibits a complex phase diagram with multiple superconducting states, yet the nature of their coexistence has remained a central mystery. In particular, the apparent intersection of two second-order phase boundaries at a “triple point” in the pressure-temperature phase diagram is thermodynamically forbidden, suggesting hidden phase […]

Kavli Affiliate: Brad Ramshaw | Summary:The candidate topological superconductor UTe$_2$ exhibits a complex phase diagram with multiple superconducting states, yet the nature of their coexistence has remained a central mystery. In particular, the apparent intersection of two second-order phase boundaries at a “triple point” in the pressure-temperature phase diagram is thermodynamically forbidden, suggesting either hidden […]

Kavli Affiliate: Darrell Schlom | Summary:Mesoscopic transport measurements are underexplored as probes of quasiparticles and their properties in correlated metals. The mixed valence compound YbAl$_3$ exhibits a single-ion Kondo temperature of 670 K, while thermodynamic and transport properties (probed with specific heat, magnetic susceptibility, Hall effect, and resistivity) imply the onset of coherence of heavy […]

Kavli Affiliate: David Muller | Summary:We present Kamino, a GPU-based physics solver for massively parallel simulations of heterogeneous highly-coupled mechanical systems. Implemented in Python using NVIDIA Warp and integrated into the Newton framework, it enables the application of data-driven methods, such as large-scale reinforcement learning, to complex robotic systems that exhibit strongly coupled kinematic and […]

Kavli Affiliate: Richard D. Robinson | Summary:Achieving large optical rotation with minimal ellipticity and absorption, ‘pure’ optical rotation, remains a central challenge in chiral photonics. Solution-processed self-assembled materials can exhibit exceptional chiroptical responses (g-factors > 1), yet their circular birefringence (CB) typically overlaps with circular dichroism (CD) and resonant loss (Absorption), leading to elliptical, attenuated […]

Kavli Affiliate: David Muller | Summary:How ordered phases melt in low-dimensional quantum materials remain difficult to resolve because the relevant fluctuations are dynamic and charge neutral. In this work, we show that thermal transport provides a sensitive probe of these hidden fluctuations in the layered transition metal dichalcogenide 2H-TaSe2. We observe a striking V-shaped temperature […]