Kavli Affiliate: Darrell Schlom | Summary:The prototypical Mott-Hubbard insulator LaVO3 undergoes a structural phase transition accompanied by the onset of spin and orbital ordering below 140 K. By combining ultrafast optical pump-probe spectroscopy and two-dimensional electronic spectroscopy, we investigate the interplay between fluctuations of the local spin and orbital order parameter and the lifetime of […]
Continue.. Tracking the local order parameter through the Hubbard exciton decoherence time in the Mott-Hubbard insulator LaVO3