Kavli Affiliate: Birgitta Whaley
| First 5 Authors: Vladislav Yu. Shishkov, Evgeny S. Andrianov, Sergei Tretiak, K. Birgitta Whaley, Anton V. Zasedatelev
| Summary:
We demonstrate a macro-coherent regime in exciton-polariton systems, where
nonequilibrium polariton Bose–Einstein condensation coexists with
macroscopically occupied vibrational states. Strong exciton-vibration coupling
induces an effective optomechanical interaction between cavity polaritons and
vibrational degrees of freedom of molecules, leading to vibrational
amplification in a resonant blue-detuned configuration. This interaction
provide a sympathetic mechanism to achieve vibrational condensation with
potential applications in cavity-controlled chemistry, nonlinear and quantum
optics.
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